[@Polaris North] The third option would be for her to listen in on Kent's Silver Shroud broadcasts and decide that Goodneighbour has a fellow defender of justice active there. She might make an attempt to try and meet up with the hero to try and form 'The New Unstoppables'.

She might be a little unhappy if she finds out the Silver Shroud isn't real, unless someone tries to trick her into helping Goodneighbour instead of slaughtering everyone in the neighbourhood. This could offer Hancock another source of 'security' for his expension plans, rather than relying on the Triggermen.
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If she does feel the want to visit Goodneighbor, I think it's pretty painfully obvious just how... 'chaotic' it is. But really, isn't her kind of peacekeeping the same as Hancock's in that regard? But yeah, relying on the Triggermen is one of the problems right now so it might be a good idea to have an allegiance with her. Though it is up to you if you want or not.